Physical constrains and functional plasticity of cellulases: Linear scaling relationships for a heterogeneous enzyme reaction
J. Kari, G. Molina, K. Schaller, S. Christensen, C. Schiano-di-Cola, S. Badino, T. Soerensen, N. Roejel, M. Keller, B. Kolaczkowski, J. P. Olsen, K. Krogh, K. Jensen, A. M. Cavaleiro, G. H. Peters, , P. Westh
The paper characterizes 83 cellulases, revealing a linear free energy relationship between substrate binding strength and activation barrier, suggesting physical constraints and evolutionary optimization in interfacial enzyme catalysis.
bioRxiv · May 20, 2020 · PreprintBiochemistry